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Tekirdağ iline içme suyu sağlayan bazı baraj gölü/gölet yüzey sedimanlarında PAH, PCB ve OCP düzeylerinin belirlenmesi ve risk değerlendirmesi

Year 2022, Volume: 37 Issue: 3, 1453 - 1468, 28.02.2022

Oltan Canlı

https://doi.org/10.17341/gazimmfd.953925

Abstract

Bu çalışmada, Tekirdağ iline içme suyu sağlayan bazı baraj gölü/göletlerin yüzey sedimanlarında bazı organik kirleticilerinin (PAH, PCB ve OCP) seviyesini ortaya koymak, olası PAH kaynaklarını belirlemek ve sediman kalitesinin ekolojik risk değerlendirmesi ile amaçlanmıştır. Yüzey sediman örnekleri Ekim 2020’ de Naipköy barajı, Türkmenli Göleti, Yazır Göleti ve Şarköy Göletinden alınmıştır. Örneklerin PAH, PCB ve OCP konsantrasyonları GC-MS/MS kullanılarak ölçülmüştür. Örneklerdeki toplam PAH konsantrasyonları 20,56 ng/g (T5) ile 124,4 ng/g (T4) arasında değişmektedir. Örnekler bireysel PAH bileşikleri bakımından incelendiğinde, sırasıyla Naftalen, Fenantren, Floranten, Piren, Benzo(b)floranten, Krizen ve Floren baskın PAH bileşikleridir. T2 sediman örneği hariç, diğer tüm sediman örneklerinde Naftalen baskın durumdadır ve konsantrasyonu 6,929 ng/g (T2) ile 72,67 ng/g (T4) aralığından tespit edilmiştir. Toplam OCP konsantrasyonu 0,710 ng/g (T5) -7,918 ng/g (T8) aralığında değişirken, toplam PCB konsantrasyonu 0,120 ng/g (T5) -0,383 (T8) ng/g aralığında bulunmuştur. Örneklerde en baskın OCP bileşikleri sırasıyla DDT p,p, DDE p,p ve HCH alfa olurken, aynı örneklerde PCB 153, 138 ve 180 en yüksek tespit edilen PCB konjeneleridirler. PAH'ların kaynak tanımlaması PAH bileşiklerinin moleküler oranları kullanılarak yapılmıştır. Hesaplanan tüm moleküler oranlar bir arada düşündüğünde, sediman örneklerindeki PAH bileşiklerinin kaynağının daha çok petrojenik kaynaklı olduğu bulunmuştur. Örneklerdeki PAH, PCB ve OCP'lerin seviyelerinin hiçbiri, su organizmalarında toksik etkilerin sıklıkla meydana geldiği kirletici seviyesi olan ERM değerlerini geçmemiştir.

Keywords

yüzey sediman risk değerlendirmesi PAH PCB OCP

Supporting Institution

Yok

Project Number

Yok

Thanks

Yazar, PAH, PCB ve OCP'lerin analizi, sediman örneklerinin ön işlemleri ve makale yazım aşamasında sağladıkları sonsuz destek, nazik öneriler ve yardımları için Beyza YÜCE, Ertuğrul ASLAN ve Barış GÜZEL'e teşekkür eder.

References

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Year 2022, Volume: 37 Issue: 3, 1453 - 1468, 28.02.2022

Oltan Canlı

https://doi.org/10.17341/gazimmfd.953925

Abstract

Project Number

Yok

References

  • 1. Botwe B.O., Kelderman P., Nyarko E., Lens P.N.L., Assessment of DDT, HCH and PAH Contamination and Associated Ecotoxicological Risks in Surface Sediments of Coastal Tema Harbour (Ghana), Mar. Pollut. Bull. 115, 480-488, 2017.
  • 2. Kanzari F., Syakti A.G., Asia L., Malleret L., Mille G., Jamoussi B., Abderrabba M., Doumenq P., Aliphatic Hydrocarbons, Polycyclic Aromatic Hydrocarbons, Polychlorinated Biphenyls, Organochlorine, And Organophosphorous Pesticides in Surface Sediments from The Arc River and The Berre Lagoon, France, Environ. Sci. Pollut. Res., 19, 559-576, 2012.
  • 3. Başar H., Güzel B., Özer Erdoğan P., Tolun L., Determination of The Environmental Effects of Turkey's Marine Dredged Materials Prior To Beneficial Use: Commercial Ports & Fishery Harbours, J. Fac. Eng. Archit. Gaz., 32 (4), 1063-1076, 2017.
  • 4. Bersuder P., Smith A.J., Hynes C., Warford L., Barber J.L., Losada S., Limpenny C., Khamis A.S., Abdulla K.H., Le Quesne W.J.F., Lyons B.P., Baseline Survey of Marine Sediments Collected from The Kingdom of Bahrain: PAHs, PCBs, Organochlorine Pesticides, Perfluoroalkyl Substances, Dioxins, Brominated Flame Retardants and Metal Contamination, Mar. Pollut. Bull., 161, 111734, 2020.
  • 5. Guzel B., Basar H.M., Gunes K., Yenisoy-Karakas S. Tolun L., Investigation of Topsoil Production from Marine Dredged Materials (DMs) In Turkey for Urban Landscaping Works, Heliyon, 5 (7), e0213, 2019.
  • 6. Yılmaz A., Tolun L., Okay O.S., Pollution and Toxicity of Sediment in Potential Dredging Sites of the Marmara Sea, Turkey, J. Environ. Sci. and Health, Part A, 54 (12), 1206-1218, 2019.
  • 7. Akdemir T., Dalgic G., The impact of the Marine Sewage Outfalls On the Sediment Quality: The Black Sea and The Marmara Case, Saudi J. Biol. Sci., 28 (1), 238-246, 2021.
  • 8. Başar H., Güzel B., Özer-erdoğan P., Murat-Hocaoğlu S., Özel D., Ergenekon Ş., Tolun G., Deniz Dibi Tarama Malzemesinin Faydalı Kullanımı için Yıkama-Eleme Tesisi Tasarımı ve Yıkama-Eleme Prosesi Atıksuyunun Yönetimi, Sakarya Uni. J. Sci., 22 (2), 735-747, 2018.
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  • 11. Warner J., Osuch J.R., Karmaus W., Landgraf J.R., Taffe B., O’Keefe M., Mikucki D., Haan P., Common Classification Schemes for PCB Congeners and The Gene Expression of CYP17, CYP19, ESR1 and ESR2, Sci. Total Environ., 414, 81–89, 2012.
  • 12. Mitra S., Corsolini S., Pozo K., Audy O., Sarkar S.K., Biswas J.K., Characterization, Source Identification and Risk Associated with Polyaromatic and Chlorinated Organic Contaminants (PAHs, PCBs, PCBzs and OCPs) in The Surface Sediments of Hooghly Estuary, India, Chemosphere, 221, 154-165, 2019.
  • 13. Erkul Ş., Eker Şanlı G., Determination of Polychlorinated Biphenyl (PCB) Concentrations of Olive Groves in Spring Season. J. Fac. Eng. Archit. Gaz., 35 (2), 1003-1014, 2020.
  • 14. Wang X., Chen L., Wang X., Lei B., Sun Y., Zhou J., Wu M., Occurrence, Sources and Health Risk Assessment of Polycyclic Aromatic Hydrocarbons in Urban (Pudong) and Suburban Soils from Shanghai in China, Chemosphere 119, 1224-1232, 2015.
  • 15. Eker G. Spatial Variations of Polycyclic Aromatic Hydrocarbons (PAHs) Concentrations in Olive Grove Area Soils in Bursa, J. Fac. Eng. Archit. Gaz., 32 (2), 607-616, 2017.
  • 16. Zhao Z., Jiang Y., Li Q., Cai Y., Hongbin Y., Zhang L., Zhang J., Spatial Correlation Analysis of Polycyclic Aromatic Hydrocarbons (PAHs) and Organochlorine Pesticides (OCPs) in Sediments Between Taihu Lake and Its Tributary Rivers, Ecotoxicol. Environ. Saf., 142, 117-128, 2017.
  • 17. Rabodonirina S., Net S., Ouddane B., Merhaby D., Dumoulin D., Popescu T., Ravelonandro P., Distribution of Persistent Organic Pollutants (PAHs, MePAHs, PCBs) in Dissolved, Particulate and Sedimentary Phases in Freshwater Systems, Environ. Pollut., 206, 38–48, 2015.
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  • 19. Choi H.G., Moon H.B., Choi M., Yu J. Monitoring of Organic Contaminants in Sediments from The Korean Coast: Spatial Distribution and Temporal Trends (2001–2007), Mar. Pollut. Bull., 62, 1352–1361, 2011.
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  • 24. Shrivastava A., Gupta V.B., Methods for the Determination of Limit of Detection and Limit of Quantitation of the Analytical Methods, Chron. Young Sci., 2, 21-25, 2011.
  • 25. Güzel B., Canlı O. Method Validation and Measurement Uncertainty of Possible Thirty Volatile Organic Compounds (VOCs) Presented in the Polyethylene Present in Bottled Drinking Waters Sold in Turkey, J. Anal. Sci. & Tech., 11 (44), 1-17, 2020.
  • 26. Güzel B., Canlı O., Öktem Olgun E, Gas Chromatography Method Validation Study for Sensitive and Accurate Determination of Volatile Aromatic Hydrocarbons (VAHs) in Water. Cumhuriyet Sci. J., 39 (4), 970-982, 2018.
  • 27. Güzel B., Canlı O., Applicability of Purge and Trap Gas Chromatography-Mass Spectrometry Method for Sensitive Analytical Detection of Naphthalene and Its Derivatives in Waters, J. Mass Spectrom., 55, e4672, 2020.
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There are 59 citations in total.

Details

Primary Language Turkish
Subjects Engineering
Journal Section Makaleler
Authors

Oltan Canlı 0000-0002-2652-844X

Project Number Yok
Publication Date February 28, 2022
Submission Date June 18, 2021
Acceptance Date October 6, 2021
Published in Issue Year 2022 Volume: 37 Issue: 3

Cite

APA Canlı, O. (2022). Tekirdağ iline içme suyu sağlayan bazı baraj gölü/gölet yüzey sedimanlarında PAH, PCB ve OCP düzeylerinin belirlenmesi ve risk değerlendirmesi. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi, 37(3), 1453-1468. https://doi.org/10.17341/gazimmfd.953925
AMA Canlı O. Tekirdağ iline içme suyu sağlayan bazı baraj gölü/gölet yüzey sedimanlarında PAH, PCB ve OCP düzeylerinin belirlenmesi ve risk değerlendirmesi. GUMMFD. February 2022;37(3):1453-1468. doi:10.17341/gazimmfd.953925
Chicago Canlı, Oltan. “Tekirdağ Iline içme Suyu sağlayan Bazı Baraj gölü/Gölet yüzey sedimanlarında PAH, PCB Ve OCP düzeylerinin Belirlenmesi Ve Risk değerlendirmesi”. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi 37, no. 3 (February 2022): 1453-68. https://doi.org/10.17341/gazimmfd.953925.
EndNote Canlı O (February 1, 2022) Tekirdağ iline içme suyu sağlayan bazı baraj gölü/gölet yüzey sedimanlarında PAH, PCB ve OCP düzeylerinin belirlenmesi ve risk değerlendirmesi. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi 37 3 1453–1468.
IEEE O. Canlı, “Tekirdağ iline içme suyu sağlayan bazı baraj gölü/gölet yüzey sedimanlarında PAH, PCB ve OCP düzeylerinin belirlenmesi ve risk değerlendirmesi”, GUMMFD, vol. 37, no. 3, pp. 1453–1468, 2022, doi: 10.17341/gazimmfd.953925.
ISNAD Canlı, Oltan. “Tekirdağ Iline içme Suyu sağlayan Bazı Baraj gölü/Gölet yüzey sedimanlarında PAH, PCB Ve OCP düzeylerinin Belirlenmesi Ve Risk değerlendirmesi”. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi 37/3 (February 2022), 1453-1468. https://doi.org/10.17341/gazimmfd.953925.
JAMA Canlı O. Tekirdağ iline içme suyu sağlayan bazı baraj gölü/gölet yüzey sedimanlarında PAH, PCB ve OCP düzeylerinin belirlenmesi ve risk değerlendirmesi. GUMMFD. 2022;37:1453–1468.
MLA Canlı, Oltan. “Tekirdağ Iline içme Suyu sağlayan Bazı Baraj gölü/Gölet yüzey sedimanlarında PAH, PCB Ve OCP düzeylerinin Belirlenmesi Ve Risk değerlendirmesi”. Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi, vol. 37, no. 3, 2022, pp. 1453-68, doi:10.17341/gazimmfd.953925.
Vancouver Canlı O. Tekirdağ iline içme suyu sağlayan bazı baraj gölü/gölet yüzey sedimanlarında PAH, PCB ve OCP düzeylerinin belirlenmesi ve risk değerlendirmesi. GUMMFD. 2022;37(3):1453-68.