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Experimental Study on The Gamma Ray Absorption Properties of Lanthanum and Cerium Borides

Year 2023, Volume: 18 Issue: 3, 238 - 247, 23.11.2023
https://doi.org/10.29233/sdufeffd.1355393

Abstract

The objective of this study is to investigate the mass attenuation coefficients (μm) of lanthanumhexaborides and ceriumhexaborides over a wide photon energy range emitted from the main radioactive sources used in medicine and industry. 125I, 99mTc, 131I, 137Cs, 60Co and 152Eu gamma ray sources were used in the experiments. The materials synthesized in powder form were first pelletized and then irradiated by photon beams. At the end, it was seen that there is successful consistency between the obtained experimental data and the previous theoretical results. It was also observed that the investigated samples are comparable enough to the known standard gamma shielding materials, especially to lead which is one of the most common one. In conclusion, it is understood that the presently investigated samples have a promising aspect in terms of developing new shielding materials against gamma rays.

References

  • R. Kurtulus, C. Kurtulus and T. Kavas, “Nuclear radiation shielding characteristics and physical, optical, mechanical, and thermal properties of lithium-borotellurite glass doped with Rb2O”, Progress in Nuclear Energy, 141, 103961, 2021.
  • K. G. Mahmoud, M. I. Sayyed, D. A. Aloraini, A. H. Almuqrin and A. S. Abouhaswa, “. Impacts of praseodymium (III, IV) oxide on physical, optical, and gamma-ray shielding properties of boro-silicate glasses”, Radiation Physics and Chemistry, 207, 110836, 2023.
  • A. Şengül, I. Akkurt, K. Gunoglu, K. Akgüngör and R. B. Ermis, “Experimental evaluation of gamma-rays shielding properties of ceramic materials used in dentistry”, Radiation Physics and Chemistry, 204, 110701, 2023.
  • S. Dezhampanah, I. M. Nikbin, S. Mehdipour, R. Mohebbi and H. H. Moghadam, “Fiber- reinforced concrete containing nano - TiO2 as a new gamma-ray radiation shielding materials”, Journal of Building Engineering, 44, 102542, 2021.
  • S. Kumar, K. S. Mann, T. Singh and S. Singh, “Investigations on the gamma-ray shielding performance of green concrete using theoretical, experimental and simulation techniques”, Progress in Nuclear Energy, 134, 103654, 2021.
  • F. H. Sallam, M. Tharwat, A. H. Almuqrin, M. I. Sayyed and K. A. Mahmoud, “Ni0.5Zn0.5Fe2O4 nanoparticles reinforced polyester composite for advanced radiation shielding applications: A detailed discussion for synthesis, characterization, and gamma-ray attenuation properties”, Radiation Physics and Chemistry, 208, 110907, 2023.
  • M. Elsafi, H. Al-Ghamdi, M. I. Sayyed, A. Antar, A. H. Almuqrin, K. A. Mahmoud, K. Cornish, T. I. Shalaby and A. M. El-Khatib, “Optimizing the gamma-ray shielding behaviors for polypropylene using lead oxide: a detailed examination”, Journal of Materials Research and Technology, 19, 1862-1872, 2022.
  • J. H. Hubbell, “Photon Mass Attenuation and Energy-Absorption Coefficients”, The International Journal Of Applied Radiation And Isotopes, 33(11),1269–90, 1982.
  • I. Akkurt, H. Akyıldırım, B. Mavi, S. Kilincarslan and C. Basyigit. “Photon Attenuation Coefficients of Concrete Includes Barite in Different Rate”, Annals of Nuclear Energy, 37(7), 910–14, 2010.
  • C. Eke, O. Agar, C. Segebade and I. Boztosun, “Attenuation Properties of Radiation ShieldingMaterials Such as Granite and Marble against γ-Ray Energies between 80 and 1350 KeV”, Radiochimica Acta, 105(10), 851–63, 2017.
  • J. Majid and A. Mohammadi, “Gamma Ray Attenuation Coefficient Measurement for Neutron-Absorbent Materials”, Radiation Physics and Chemistry, 77(5), 523–27, 2008.
  • R. McCuen, “Book Reviews”, JAWRA Journal of the American Water Resources Association, 48(2), 407–10, 2012.
  • J. M. Sharaf and M. S. Hamideen, “Photon Attenuation Coefficients and Shielding Effects of Jordanian Building Materials”, Annals of Nuclear Energy, 62, 50–56, 2013.
  • G. C. Jagetia, “Radioprotective Potential of Plants and Herbs against the Effects of Ionizing Radiation”, Journal of Clinical Biochemistry and Nutrition, 40(2), 74–81, 2007.
  • Y. Karabul, L. A. Susam, O. Içelli and Ö. Eyecioǧlu, “Computation of EABF and EBF for Basalt Rock Samples”, Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, 797, 29–36, 2015.
  • M. Çağlar, H. Kayacık, Y. Karabul, M. Kılıç, Z. G. Özdemir and O. İçelli, “Na2Si3O7/BaO Composites for the Gamma-Ray Shielding in Medical Applications: Experimental, MCNP5, and WinXCom Studies”, Progress in Nuclear Energy, 117, 103-119, 2019.
  • K. Ashok, “Gamma Ray Shielding Properties of PbO-Li2O-B2O3 Glasses”, Radiation Physics and Chemistry, 136, 50–53, 2017.
  • A. Nigar, Z. Yüksel, E. Abbasov, H. Gülbiçim and M. Ç. Tufan, “Investigation of Gamma-Ray Attenuation Parameters of Some Materials Used in Dental Applications”, Results in Physics, 12, 2202–2205, 2019.
  • A. Hakan, “Olivine Mineral Used inConcrete for Gamma-Ray Shielding”, Arabian Journal of Geosciences, 12(8), 1–8, 2019.
  • M. Asghar and H. Ghiasi, “Shielding Properties of the Ordinary Concrete Loaded with Micro-and Nano-Particles against Neutron and Gamma Radiations”, Applied Radiation and Isotopes, 136, 27–31, 2018.
  • H. O. Tekin, M. I. Sayyed, E. E. Altunsoy and T. Manici, “Shielding Properties and Effects of WO3 and PbO on Mass Attenuation Coefficients by Using MCNPX Code”, Digest Journal of Nanomaterials and Biostructures, 12(3), 861–67, 2017.
  • M. G. Dong, M. I. Sayyed, G. Lakshminarayana, M. Çelikbilek, A. E. Ersundu, P. Nayar and M. A. Mahdi, “Investigation of Gamma Radiation Shielding Properties of Lithium Zinc Bismuth Borate Glasses Using XCOM Program and MCNP5 Code”, Journal of Non-Crystalline Solids, 468, 12–16, 2017.
  • Z. Li, W. Zhou, X. Zhang, Y. Gao and S. Guo, S., “High-efficiency, flexibility and lead-free X-ray shielding multilayered polymer composites: layered structure design and shielding mechanism”, Scientific Reports, 11, 4384, 2021.
  • Y. Kavun, S. Kerli, H. Eskalen and M. Kavgacı, “Characterization and nuclear shielding performance of Sm doped In₂O thin films”, Radiation Physics and Chemistry, 194, 110014, 2022.
  • M. Alqahtani, F. Ercan, N. A. Saleh, M. H. A. Mhareb, N. Dwaikat, M. I. Sayyed, F. Abokhamis, A. Abdulrazzaq, B. Ozcelik and I. Ercan, “Structural, magnetic and gamma-ray shielding features of Zn doped Mg2FeTiO6 double perovskite”, Physica B Condensed Matter, 640, 414024, 2022.
  • H. Yaykaslı, H. Eskalen, Y. Kavun and M. Gögebakan “Microstructural, thermal, and radiation shielding properties of Al50B25Mg25 alloy prepared by mechanical alloying”, Journal of Materials Science: Materials in Electronics, 33, 2350–2359, 2022.
  • H. Eskalen, Y. Kavun, S. Kerli and S. Eken, “An investigation of radiation shielding properties of boron doped ZnO thin films”, Optical Materials, 105, 109871, 2020.
  • Y. Kavun, H. Eskalen, S. Kerli and M. Kavgaci, “Fabrication and characterization of GdxFe2O3 (100-x)/PVA (x= 0, 5, 10, 20) composite films for radiation shielding”, Applied Radiation and Isotopes, 177, 109918, 2021.
  • M. I. Sayyed, O. Agar, A. Kumar, H. O. Tekin, D. K. Gaikwad and S. S. Obaid, “Shielding behaviour of (20+ x) Bi2O3–20BaO–10Na2O–10MgO–(40–x) B2O3: An experimental and Monte Carlo study”, Chemical Physics, 529, 110571, 2020.
  • Y. Kavun, H. Eskalen and M. Kavgacı, “A study on gamma radiation shielding performance and characterization of graphitic carbon nitride”, Chemical Physics Letters, 811, 140246, 2023.
  • M. Elsafi, M. A. El-Nahal, M. I. Sayyed, I. H. Saleh and M. I. Abbas, “Effect of bulk and nanoparticle Bi2O3 on attenuation capability of radiation shielding glass”, Ceramics International, 47, 19651–19658, 2021.
  • M. A. El-Nahal, M. Elsafi, M. I. Sayyed, M.U. Khandaker, H. Osman, B. H. Elesawy, I. H. Saleh and M. I. Abbas, “Understanding the effect of introducing micro-and nanoparticle bismuth oxide (Bi2O3) on the gamma ray shielding performance of novel concrete”, Materials, 14(21), 6487, 2021.
  • A. Khan, A. Al-Alhareth, S. Mobark, W. Al-Mahri, N. Al-Sharyah, S. Al-Zmanan, H. B. Albargi and A. M. Abdalla, A.M., “Experimental and theoretical investigations of the γ-rays shielding performance of rock samples from Najran region”, Annals of Nuclear Energy, 183, 109676, 2023.
  • R. Arya, R. Paulose, V. Agrawal, A. Pandey, D. Mishra, S. K. Sanghi and S. T. Salammal, “Next generation gamma ray shielding blocks developed using alumina industry waste”, Construction and Building Materials, 373, 130895, 2023.
  • N. Ekinci, F. I. El-Agawany, A Gurol, Y. S. Rammah, E. M. Ahmed, D. Yılmaz, B. Aygün and M. Somer, “Physical properties, experimental and theoretical gamma-ray shielding”, Radiation Physics and Chemistry, 194, 110012, 2022.
  • H. Gulbicim, M. N. Turkan, M. Aksu and S. Durmuş, “A study on the investigation of gamma shielding properties of some metal borides”, Progress in Nuclear Energy, 115, 107–114, 2019.
  • A. Özcan, M. N. Türkan, M. Aksu, H. Gülbiçim and E. Kurt, “Magnezyotermik indirgeme ile sentezlenen Lantanyum hekzaborür (LaB6) ve Seryum hekzaborür (CeB6) malzemelerinin gama zırhlama özelliklerinin Monte Carlo simülasyonu”, Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi, 38(2), 927-936, 2023.
  • Y. Wang, K. C. Chou and G. H. Zhang, “Preparations of lanthanum hexaboride (LaB6) and cerium hexaboride (CeB6)”, Journal of the American Ceramic Society, 105(3), 1954-1966, 2022.
  • H. Gülbiçim, M. Ç. Tufan and M. N. Türkan, “The investigation of vermiculite as an alternating shielding material for gamma rays”, Radiation Physics and Chemistry, 130, 112-117, 2017.
  • D. Ickecan, M. N. Turkan and H. Gulbi̇cim, “Investigation of shielding properties of impregnated activated carbon for gamma-rays”, Applied Radiation and Isotopes, 172, 109687, 2021.
Year 2023, Volume: 18 Issue: 3, 238 - 247, 23.11.2023
https://doi.org/10.29233/sdufeffd.1355393

Abstract

References

  • R. Kurtulus, C. Kurtulus and T. Kavas, “Nuclear radiation shielding characteristics and physical, optical, mechanical, and thermal properties of lithium-borotellurite glass doped with Rb2O”, Progress in Nuclear Energy, 141, 103961, 2021.
  • K. G. Mahmoud, M. I. Sayyed, D. A. Aloraini, A. H. Almuqrin and A. S. Abouhaswa, “. Impacts of praseodymium (III, IV) oxide on physical, optical, and gamma-ray shielding properties of boro-silicate glasses”, Radiation Physics and Chemistry, 207, 110836, 2023.
  • A. Şengül, I. Akkurt, K. Gunoglu, K. Akgüngör and R. B. Ermis, “Experimental evaluation of gamma-rays shielding properties of ceramic materials used in dentistry”, Radiation Physics and Chemistry, 204, 110701, 2023.
  • S. Dezhampanah, I. M. Nikbin, S. Mehdipour, R. Mohebbi and H. H. Moghadam, “Fiber- reinforced concrete containing nano - TiO2 as a new gamma-ray radiation shielding materials”, Journal of Building Engineering, 44, 102542, 2021.
  • S. Kumar, K. S. Mann, T. Singh and S. Singh, “Investigations on the gamma-ray shielding performance of green concrete using theoretical, experimental and simulation techniques”, Progress in Nuclear Energy, 134, 103654, 2021.
  • F. H. Sallam, M. Tharwat, A. H. Almuqrin, M. I. Sayyed and K. A. Mahmoud, “Ni0.5Zn0.5Fe2O4 nanoparticles reinforced polyester composite for advanced radiation shielding applications: A detailed discussion for synthesis, characterization, and gamma-ray attenuation properties”, Radiation Physics and Chemistry, 208, 110907, 2023.
  • M. Elsafi, H. Al-Ghamdi, M. I. Sayyed, A. Antar, A. H. Almuqrin, K. A. Mahmoud, K. Cornish, T. I. Shalaby and A. M. El-Khatib, “Optimizing the gamma-ray shielding behaviors for polypropylene using lead oxide: a detailed examination”, Journal of Materials Research and Technology, 19, 1862-1872, 2022.
  • J. H. Hubbell, “Photon Mass Attenuation and Energy-Absorption Coefficients”, The International Journal Of Applied Radiation And Isotopes, 33(11),1269–90, 1982.
  • I. Akkurt, H. Akyıldırım, B. Mavi, S. Kilincarslan and C. Basyigit. “Photon Attenuation Coefficients of Concrete Includes Barite in Different Rate”, Annals of Nuclear Energy, 37(7), 910–14, 2010.
  • C. Eke, O. Agar, C. Segebade and I. Boztosun, “Attenuation Properties of Radiation ShieldingMaterials Such as Granite and Marble against γ-Ray Energies between 80 and 1350 KeV”, Radiochimica Acta, 105(10), 851–63, 2017.
  • J. Majid and A. Mohammadi, “Gamma Ray Attenuation Coefficient Measurement for Neutron-Absorbent Materials”, Radiation Physics and Chemistry, 77(5), 523–27, 2008.
  • R. McCuen, “Book Reviews”, JAWRA Journal of the American Water Resources Association, 48(2), 407–10, 2012.
  • J. M. Sharaf and M. S. Hamideen, “Photon Attenuation Coefficients and Shielding Effects of Jordanian Building Materials”, Annals of Nuclear Energy, 62, 50–56, 2013.
  • G. C. Jagetia, “Radioprotective Potential of Plants and Herbs against the Effects of Ionizing Radiation”, Journal of Clinical Biochemistry and Nutrition, 40(2), 74–81, 2007.
  • Y. Karabul, L. A. Susam, O. Içelli and Ö. Eyecioǧlu, “Computation of EABF and EBF for Basalt Rock Samples”, Nuclear Instruments and Methods in Physics Research, Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, 797, 29–36, 2015.
  • M. Çağlar, H. Kayacık, Y. Karabul, M. Kılıç, Z. G. Özdemir and O. İçelli, “Na2Si3O7/BaO Composites for the Gamma-Ray Shielding in Medical Applications: Experimental, MCNP5, and WinXCom Studies”, Progress in Nuclear Energy, 117, 103-119, 2019.
  • K. Ashok, “Gamma Ray Shielding Properties of PbO-Li2O-B2O3 Glasses”, Radiation Physics and Chemistry, 136, 50–53, 2017.
  • A. Nigar, Z. Yüksel, E. Abbasov, H. Gülbiçim and M. Ç. Tufan, “Investigation of Gamma-Ray Attenuation Parameters of Some Materials Used in Dental Applications”, Results in Physics, 12, 2202–2205, 2019.
  • A. Hakan, “Olivine Mineral Used inConcrete for Gamma-Ray Shielding”, Arabian Journal of Geosciences, 12(8), 1–8, 2019.
  • M. Asghar and H. Ghiasi, “Shielding Properties of the Ordinary Concrete Loaded with Micro-and Nano-Particles against Neutron and Gamma Radiations”, Applied Radiation and Isotopes, 136, 27–31, 2018.
  • H. O. Tekin, M. I. Sayyed, E. E. Altunsoy and T. Manici, “Shielding Properties and Effects of WO3 and PbO on Mass Attenuation Coefficients by Using MCNPX Code”, Digest Journal of Nanomaterials and Biostructures, 12(3), 861–67, 2017.
  • M. G. Dong, M. I. Sayyed, G. Lakshminarayana, M. Çelikbilek, A. E. Ersundu, P. Nayar and M. A. Mahdi, “Investigation of Gamma Radiation Shielding Properties of Lithium Zinc Bismuth Borate Glasses Using XCOM Program and MCNP5 Code”, Journal of Non-Crystalline Solids, 468, 12–16, 2017.
  • Z. Li, W. Zhou, X. Zhang, Y. Gao and S. Guo, S., “High-efficiency, flexibility and lead-free X-ray shielding multilayered polymer composites: layered structure design and shielding mechanism”, Scientific Reports, 11, 4384, 2021.
  • Y. Kavun, S. Kerli, H. Eskalen and M. Kavgacı, “Characterization and nuclear shielding performance of Sm doped In₂O thin films”, Radiation Physics and Chemistry, 194, 110014, 2022.
  • M. Alqahtani, F. Ercan, N. A. Saleh, M. H. A. Mhareb, N. Dwaikat, M. I. Sayyed, F. Abokhamis, A. Abdulrazzaq, B. Ozcelik and I. Ercan, “Structural, magnetic and gamma-ray shielding features of Zn doped Mg2FeTiO6 double perovskite”, Physica B Condensed Matter, 640, 414024, 2022.
  • H. Yaykaslı, H. Eskalen, Y. Kavun and M. Gögebakan “Microstructural, thermal, and radiation shielding properties of Al50B25Mg25 alloy prepared by mechanical alloying”, Journal of Materials Science: Materials in Electronics, 33, 2350–2359, 2022.
  • H. Eskalen, Y. Kavun, S. Kerli and S. Eken, “An investigation of radiation shielding properties of boron doped ZnO thin films”, Optical Materials, 105, 109871, 2020.
  • Y. Kavun, H. Eskalen, S. Kerli and M. Kavgaci, “Fabrication and characterization of GdxFe2O3 (100-x)/PVA (x= 0, 5, 10, 20) composite films for radiation shielding”, Applied Radiation and Isotopes, 177, 109918, 2021.
  • M. I. Sayyed, O. Agar, A. Kumar, H. O. Tekin, D. K. Gaikwad and S. S. Obaid, “Shielding behaviour of (20+ x) Bi2O3–20BaO–10Na2O–10MgO–(40–x) B2O3: An experimental and Monte Carlo study”, Chemical Physics, 529, 110571, 2020.
  • Y. Kavun, H. Eskalen and M. Kavgacı, “A study on gamma radiation shielding performance and characterization of graphitic carbon nitride”, Chemical Physics Letters, 811, 140246, 2023.
  • M. Elsafi, M. A. El-Nahal, M. I. Sayyed, I. H. Saleh and M. I. Abbas, “Effect of bulk and nanoparticle Bi2O3 on attenuation capability of radiation shielding glass”, Ceramics International, 47, 19651–19658, 2021.
  • M. A. El-Nahal, M. Elsafi, M. I. Sayyed, M.U. Khandaker, H. Osman, B. H. Elesawy, I. H. Saleh and M. I. Abbas, “Understanding the effect of introducing micro-and nanoparticle bismuth oxide (Bi2O3) on the gamma ray shielding performance of novel concrete”, Materials, 14(21), 6487, 2021.
  • A. Khan, A. Al-Alhareth, S. Mobark, W. Al-Mahri, N. Al-Sharyah, S. Al-Zmanan, H. B. Albargi and A. M. Abdalla, A.M., “Experimental and theoretical investigations of the γ-rays shielding performance of rock samples from Najran region”, Annals of Nuclear Energy, 183, 109676, 2023.
  • R. Arya, R. Paulose, V. Agrawal, A. Pandey, D. Mishra, S. K. Sanghi and S. T. Salammal, “Next generation gamma ray shielding blocks developed using alumina industry waste”, Construction and Building Materials, 373, 130895, 2023.
  • N. Ekinci, F. I. El-Agawany, A Gurol, Y. S. Rammah, E. M. Ahmed, D. Yılmaz, B. Aygün and M. Somer, “Physical properties, experimental and theoretical gamma-ray shielding”, Radiation Physics and Chemistry, 194, 110012, 2022.
  • H. Gulbicim, M. N. Turkan, M. Aksu and S. Durmuş, “A study on the investigation of gamma shielding properties of some metal borides”, Progress in Nuclear Energy, 115, 107–114, 2019.
  • A. Özcan, M. N. Türkan, M. Aksu, H. Gülbiçim and E. Kurt, “Magnezyotermik indirgeme ile sentezlenen Lantanyum hekzaborür (LaB6) ve Seryum hekzaborür (CeB6) malzemelerinin gama zırhlama özelliklerinin Monte Carlo simülasyonu”, Gazi Üniversitesi Mühendislik Mimarlık Fakültesi Dergisi, 38(2), 927-936, 2023.
  • Y. Wang, K. C. Chou and G. H. Zhang, “Preparations of lanthanum hexaboride (LaB6) and cerium hexaboride (CeB6)”, Journal of the American Ceramic Society, 105(3), 1954-1966, 2022.
  • H. Gülbiçim, M. Ç. Tufan and M. N. Türkan, “The investigation of vermiculite as an alternating shielding material for gamma rays”, Radiation Physics and Chemistry, 130, 112-117, 2017.
  • D. Ickecan, M. N. Turkan and H. Gulbi̇cim, “Investigation of shielding properties of impregnated activated carbon for gamma-rays”, Applied Radiation and Isotopes, 172, 109687, 2021.
There are 40 citations in total.

Details

Primary Language English
Subjects Nuclear Physics
Journal Section Makaleler
Authors

Hasan Gülbiçim 0000-0003-4518-2509

Aynur Özcan 0000-0003-2514-5460

Nureddin Türkan 0000-0002-0452-9484

Mecit Aksu 0000-0002-9405-1217

Esra Kurt 0000-0001-8147-8791

Publication Date November 23, 2023
Published in Issue Year 2023 Volume: 18 Issue: 3

Cite

IEEE H. Gülbiçim, A. Özcan, N. Türkan, M. Aksu, and E. Kurt, “Experimental Study on The Gamma Ray Absorption Properties of Lanthanum and Cerium Borides”, Süleyman Demirel University Faculty of Arts and Science Journal of Science, vol. 18, no. 3, pp. 238–247, 2023, doi: 10.29233/sdufeffd.1355393.