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MONTE-CARLO (MC) ANALYSIS OF BORATED MATERIALS FOR NEUTRON SHIELDING APPLICATIONS

Year 2022, Volume: 3 Issue: 2, 63 - 70, 15.12.2022
https://doi.org/10.55696/ejset.1102371

Abstract

Neutron shielding is of utmost importance in radiation environments such as nuclear reactors and particle accelerators and in fields such as health physics. In this work, the percentages of neutrons stopped by shields comprising of boron minerals (HDPE/B2O3, Epoxy/Priceite, Epoxy/Colemanite, Epoxy/Kernite) in their composition against neutron radiation of different energies is investigated using two separate MC simulations. Different layer combinations of epoxy based borated shielding materials with HDPE sheets were then simulated to find the optimum shielding configuration. In addition, radioactivation studies were carried out for these designs. The most suitable design was found to be the layered setup of the HDPE sheet and the epoxy/colemanite composite sheet for mixed neutron energies (<1MeV).

Project Number

5190039

References

  • J.W. Shin, J.W. Lee, S. Yu, B.K., Beak J.P. Hong, Y. Seo, W.N. Kim, S.M. Hong, C.M. Koo, “Polyethylene/boron-containing composites for radiation shielding”, Thermochimica Acta, vol. 585, pp. 5-9, 10 June 2014. https://doi.org/10.1016/j.tca.2014.03.039.
  • S. T. Abdulrahman, Z. Ahmad, S. Thomas, A. A. Rahman, “Chapter 1-Introduction to neutron-shielding materials,” in Micro and Nanostructured Composite Materials for Neutron Shielding Applications, Woodhead Publishing Series in Composites Science and Engineering, pp. 1–23, 2020.
  • International Atomic Energy Agency, “NGATLAS: Atlas of Neutron Capture Cross Sections,” March 2014.
  • J.C. Sublet, A.J. Koning, D. Rochman, M. Fleming, M. Gilbert, “Delivering Both Completeness and Robustness”, In Advances in Nuclear Nonproliferation Technology and Policy Conference, Santa Fe, NM, USA. Sept. 25-30, 2015.
  • Ş.G. İrim, A.A. Wis, M.A. Kestin, O. Baykara, G. Ozkoc, A. Avcı, M. Doğru, M. Karakoç, “Physical, mechanical and neutron shielding properties of h-BN/Gd2O3/HDPE ternary nanocomposites”, Radiation Physics and Chemistry. Vol. (144), pp. 434-443. March 2018. https://doi.org/10.1016/j.radphyschem.2017.10.007.
  • CERN, "Geant4 User's Guide for Application Developers," 2016.
  • X. Campo, R. Méndez, M.A.S. Lacerda, D. Garrido, M. Embid, J. Sanz, “Experimental evaluation of neutron shielding materials”, Radiation protection dosimetry. Vol. 180, no. (1-4), pp. 382-385. 1-4-August 2018. https://doi.org/10.1093/rpd/ncx202.
  • X. Zhang, M. Yang, X. Zhang, H. Wu, S. Guo, Y. Wang, “Enhancing the neutron shielding ability of polyethylene composites with an alternating multi-layered structure”, Composites Science and Technology, vol. 150, pp. 16-23, 29 September 2017. https://doi.org/10.1016/j.compscitech.2017.06.007.
  • K. Okuno, “Neutron shielding material based on colemanite and epoxy resin”, Radiation Protection Dosimetry, vol. 115, no. 258-261, 20 December 2005. https://doi.org/10.1093/rpd/nci154.
  • F. Demir, A. Un, “Radiation Transmission of Colemanite, Tincalconite and Ulexite For 6 And 18 MV X-Rays By Using Linear Accelerator”, Applied Radiation and Isotopes, vol. 72, pp. 1-5, February 2013. https://doi.org/10.1016/j.apradiso.2012.09.020.
  • T. Korkut, A. Karabulut, G. Budak, B. Aygün, O. Gencel, A. Hançerlioğları, “Investigation Of Neutron Shielding Properties Depending On Number Of Boron Atoms For Colemanite, Ulexite And Tincal Ores By Experiments And FLUKA Monte Carlo Simulations”, Applied Radiation and Isotopes, vol. 70 no. (1), pp. 341-345, January 2012.
  • H. Binici, O. Aksogan, A.H Sevinc, A. Kucukonder, “Mechanical and Radioactivity Shielding Performances Of Mortars Made With Colemanite, Barite, Ground Basaltic Pumice And Ground Blast Furnace Slag”, Construction and Building Materials, vol. 50, pp. 177-183, 2014. https://doi.org/10.1016/j.conbuildmat.2013.09.033.
  • G. Cosansu, C. Cogun, “An İnvestigation On Use Of Colemanite Powder As Abrasive İn Abrasive Waterjet Cutting (AWJC)”, Journal Of Mechanical Science And Technology vol. 26, no. 8, pp. 2371-2380. DOI 10.1007/s12206-012-0619-9, 2012.
  • C. Kaynak, N.A. Isitman, “Synergistic Fire Retardancy of Colemanite, A Natural Hydrated Calcium Borate, ın High-İmpact Polystyrene Containing Brominated Epoxy and Antimony Oxide”, Polymer Degradation and Stability vol.96, no.5, pp.798-807, May 2011. https://doi.org/10.1016/j.polymdegradstab.2011.02.011.
  • N.A. Isitman, C. Kaynak, “Effect of Partial Substitution Of Aluminum Hydroxide With Colemanite İn Fire Retarded Low-Density Polyethylene”, Journal of Fire Sciences vol. 31, no. 1, pp. 73-84, August 2 2013. https://doi.org/10.1177/0734904112454835.
  • R. Bagheri, S.P. Shirmardi, R. Adeli, “Study on Gamma-Ray Shielding Characteristics Of Lead Oxide, Barite, And Boron Ores Using MCNP-4C Monte Carlo Code And Experimental Data”, Journal of Testing and Evaluation vol. 45, no. 6, pp. 2259-2266, 24 January 2017. DOI: 10.1520/JTE20160284.
  • K. Okuno, M. Kawai, H. Yamada, “Development Of Novel Neutron Shielding Concrete”, Nuclear Technology vol. 168 no. 2, pp. 545-552, 10 Apr 2009. https://doi.org/10.13182/NT09-A9241.
  • J. Kim, B.C. Lee, Y.V. Uhm, W. H. Miller, “Enhancement of Thermal Neutron Attenuation of Nano-B4C-BN Dispersed Neutron Shielding Polymer Nanocomposites”, Journal of Nuclear Materials vol. 453 no. 1-3, pp. 48-53, October 2014.
  • T. Özdemir, A. Güngör, A.İ. Reyhancan, “Flexible Neutron Shielding Composite Material of EPDM Rubber With Boron Trioxide: Mechanical, Thermal Investigations And Neutron Shielding Tests”, Radiation Physics and Chemistry vol. 131, pp. 7-12, February 2017. https://doi.org/10.1016/j.radphyschem.2016.10.012.
  • A.S. Kipcak, P. Gurses, E.M. Derun, N. Tugrul, S. Piskin, “Characterization of Boron Carbide Particles And İts Shielding Behavior Against Neutron Radiation”, Energy conversion and management vol. 72, pp. 39-44, August 2013. https://doi.org/10.1016/j.enconman.2012.08.026.
Year 2022, Volume: 3 Issue: 2, 63 - 70, 15.12.2022
https://doi.org/10.55696/ejset.1102371

Abstract

Supporting Institution

TÜBİTAK

Project Number

5190039

References

  • J.W. Shin, J.W. Lee, S. Yu, B.K., Beak J.P. Hong, Y. Seo, W.N. Kim, S.M. Hong, C.M. Koo, “Polyethylene/boron-containing composites for radiation shielding”, Thermochimica Acta, vol. 585, pp. 5-9, 10 June 2014. https://doi.org/10.1016/j.tca.2014.03.039.
  • S. T. Abdulrahman, Z. Ahmad, S. Thomas, A. A. Rahman, “Chapter 1-Introduction to neutron-shielding materials,” in Micro and Nanostructured Composite Materials for Neutron Shielding Applications, Woodhead Publishing Series in Composites Science and Engineering, pp. 1–23, 2020.
  • International Atomic Energy Agency, “NGATLAS: Atlas of Neutron Capture Cross Sections,” March 2014.
  • J.C. Sublet, A.J. Koning, D. Rochman, M. Fleming, M. Gilbert, “Delivering Both Completeness and Robustness”, In Advances in Nuclear Nonproliferation Technology and Policy Conference, Santa Fe, NM, USA. Sept. 25-30, 2015.
  • Ş.G. İrim, A.A. Wis, M.A. Kestin, O. Baykara, G. Ozkoc, A. Avcı, M. Doğru, M. Karakoç, “Physical, mechanical and neutron shielding properties of h-BN/Gd2O3/HDPE ternary nanocomposites”, Radiation Physics and Chemistry. Vol. (144), pp. 434-443. March 2018. https://doi.org/10.1016/j.radphyschem.2017.10.007.
  • CERN, "Geant4 User's Guide for Application Developers," 2016.
  • X. Campo, R. Méndez, M.A.S. Lacerda, D. Garrido, M. Embid, J. Sanz, “Experimental evaluation of neutron shielding materials”, Radiation protection dosimetry. Vol. 180, no. (1-4), pp. 382-385. 1-4-August 2018. https://doi.org/10.1093/rpd/ncx202.
  • X. Zhang, M. Yang, X. Zhang, H. Wu, S. Guo, Y. Wang, “Enhancing the neutron shielding ability of polyethylene composites with an alternating multi-layered structure”, Composites Science and Technology, vol. 150, pp. 16-23, 29 September 2017. https://doi.org/10.1016/j.compscitech.2017.06.007.
  • K. Okuno, “Neutron shielding material based on colemanite and epoxy resin”, Radiation Protection Dosimetry, vol. 115, no. 258-261, 20 December 2005. https://doi.org/10.1093/rpd/nci154.
  • F. Demir, A. Un, “Radiation Transmission of Colemanite, Tincalconite and Ulexite For 6 And 18 MV X-Rays By Using Linear Accelerator”, Applied Radiation and Isotopes, vol. 72, pp. 1-5, February 2013. https://doi.org/10.1016/j.apradiso.2012.09.020.
  • T. Korkut, A. Karabulut, G. Budak, B. Aygün, O. Gencel, A. Hançerlioğları, “Investigation Of Neutron Shielding Properties Depending On Number Of Boron Atoms For Colemanite, Ulexite And Tincal Ores By Experiments And FLUKA Monte Carlo Simulations”, Applied Radiation and Isotopes, vol. 70 no. (1), pp. 341-345, January 2012.
  • H. Binici, O. Aksogan, A.H Sevinc, A. Kucukonder, “Mechanical and Radioactivity Shielding Performances Of Mortars Made With Colemanite, Barite, Ground Basaltic Pumice And Ground Blast Furnace Slag”, Construction and Building Materials, vol. 50, pp. 177-183, 2014. https://doi.org/10.1016/j.conbuildmat.2013.09.033.
  • G. Cosansu, C. Cogun, “An İnvestigation On Use Of Colemanite Powder As Abrasive İn Abrasive Waterjet Cutting (AWJC)”, Journal Of Mechanical Science And Technology vol. 26, no. 8, pp. 2371-2380. DOI 10.1007/s12206-012-0619-9, 2012.
  • C. Kaynak, N.A. Isitman, “Synergistic Fire Retardancy of Colemanite, A Natural Hydrated Calcium Borate, ın High-İmpact Polystyrene Containing Brominated Epoxy and Antimony Oxide”, Polymer Degradation and Stability vol.96, no.5, pp.798-807, May 2011. https://doi.org/10.1016/j.polymdegradstab.2011.02.011.
  • N.A. Isitman, C. Kaynak, “Effect of Partial Substitution Of Aluminum Hydroxide With Colemanite İn Fire Retarded Low-Density Polyethylene”, Journal of Fire Sciences vol. 31, no. 1, pp. 73-84, August 2 2013. https://doi.org/10.1177/0734904112454835.
  • R. Bagheri, S.P. Shirmardi, R. Adeli, “Study on Gamma-Ray Shielding Characteristics Of Lead Oxide, Barite, And Boron Ores Using MCNP-4C Monte Carlo Code And Experimental Data”, Journal of Testing and Evaluation vol. 45, no. 6, pp. 2259-2266, 24 January 2017. DOI: 10.1520/JTE20160284.
  • K. Okuno, M. Kawai, H. Yamada, “Development Of Novel Neutron Shielding Concrete”, Nuclear Technology vol. 168 no. 2, pp. 545-552, 10 Apr 2009. https://doi.org/10.13182/NT09-A9241.
  • J. Kim, B.C. Lee, Y.V. Uhm, W. H. Miller, “Enhancement of Thermal Neutron Attenuation of Nano-B4C-BN Dispersed Neutron Shielding Polymer Nanocomposites”, Journal of Nuclear Materials vol. 453 no. 1-3, pp. 48-53, October 2014.
  • T. Özdemir, A. Güngör, A.İ. Reyhancan, “Flexible Neutron Shielding Composite Material of EPDM Rubber With Boron Trioxide: Mechanical, Thermal Investigations And Neutron Shielding Tests”, Radiation Physics and Chemistry vol. 131, pp. 7-12, February 2017. https://doi.org/10.1016/j.radphyschem.2016.10.012.
  • A.S. Kipcak, P. Gurses, E.M. Derun, N. Tugrul, S. Piskin, “Characterization of Boron Carbide Particles And İts Shielding Behavior Against Neutron Radiation”, Energy conversion and management vol. 72, pp. 39-44, August 2013. https://doi.org/10.1016/j.enconman.2012.08.026.
There are 20 citations in total.

Details

Primary Language English
Subjects Materials Engineering (Other)
Journal Section Research Articles
Authors

Abdulrahman Albarodi 0000-0001-6310-8658

Pelin Uslu Kiçeci 0000-0001-5271-7554

Selcen Uzun Duran 0000-0003-4943-4654

Bilge Demirköz 0000-0001-7171-5976

Project Number 5190039
Publication Date December 15, 2022
Published in Issue Year 2022 Volume: 3 Issue: 2

Cite

IEEE A. Albarodi, P. Uslu Kiçeci, S. Uzun Duran, and B. Demirköz, “MONTE-CARLO (MC) ANALYSIS OF BORATED MATERIALS FOR NEUTRON SHIELDING APPLICATIONS”, (EJSET), vol. 3, no. 2, pp. 63–70, 2022, doi: 10.55696/ejset.1102371.